1787, of written material, "dull, distasteful," from un- (1) "not" + readable (adj.). Meaning "illegible" is from 1830, but is better left to illegible.
The illegible is not plain enough to be deciphered; the unreadable is not interesting enough to be perused. [Fowler]
unquiet
unquote
unravel
unreachable
unread
unreadable
unready
unreal
unrealistic
unreality
unreason