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unharness (v.)

mid-15c., "divest of armor," from un- (2) "opposite of" + harness (v.). Similar formation in Dutch ontharnassen "to disarm." Meaning "to free (a horse) from harness" is recorded from 1610s. Related: Unharnessed; unharnessing.

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Definitions of unharness from WordNet

unharness (v.)
remove the harness from;
unharness a horse
From wordnet.princeton.edu