1530s, "hard-hearted;" 1540s, "hard, impenetrable as flint," from flint + -y (2). Literal sense of "resembling flint" is from 1640s. Related: Flintily; flintiness.
his flinty gaze
flinders
fling
flint
flint-lock
flintstone
flinty
flip
flip-flop
flippancy
flippant
flipper